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論文

Quantitative analysis of microstructure evolution, stress partitioning and thermodynamics in the dynamic transformation of Fe-14Ni alloy

Li, L.*; 宮本 吾郎*; Zhang, Y.*; Li, M.*; 諸岡 聡; 及川 勝成*; 友田 陽*; 古原 忠*

Journal of Materials Science & Technology, 184, p.221 - 234, 2024/06

 被引用回数:0 パーセンタイル:0(Materials Science, Multidisciplinary)

Dynamic transformation (DT) of austenite ($$gamma$$) to ferrite ($$alpha$$) in the hot deformation of various carbon steels was widely investigated. However, the nature of DT remains unclear due to the lack of quantitative analysis of stress partitioning between two phases and the uncertainty of local distribution of substitutional elements at the interface in multi-component carbon steels used in the previous studies. Therefore, in the present study, a binary Fe-Ni alloy with $$alpha$$+$$gamma$$ duplex microstructure in equilibrium was prepared and isothermally compressed in $$alpha$$+$$gamma$$ two-phase region to achieve quantitative analysis of microstructure evolution, stress partitioning and thermodynamics during DT. $$gamma$$ to $$alpha$$ DT during isothermal compression and $$alpha$$ to $$gamma$$ reverse transformation on isothermal annealing under unloaded condition after deformation were accompanied by Ni partitioning. The lattice strains during thermomechanical processing were obtained via in-situ neutron diffraction measurement, based on which the stress partitioning behavior between $$gamma$$ and $$alpha$$ was discussed by using the generalized Hooke's law. A thermodynamic framework for the isothermal deformation in solids was established based on the basic laws of thermodynamics, and it was shown that the total Helmholtz free energy change in the deformable material during the isothermal process should be smaller than the work done to the deformable material. Under the present thermodynamic framework, the microstructure evolution in the isothermal compression of Fe-14Ni alloy was well explained by considering the changes in chemical free energy, plastic and elastic energies and the work done to the material. In addition, the stabilization of the soft $$alpha$$ phase in Fe-14Ni alloy by deformation was rationalized since the $$gamma$$ to $$alpha$$ transformation decreased the total Helmholtz free energy by decreasing the elastic and dislocation energies.

論文

Distinguishing ion dynamics from muon diffusion in muon spin relaxation

伊藤 孝; 門野 良典*

Journal of the Physical Society of Japan, 93(4), p.044602_1 - 044602_7, 2024/04

We propose a model to describe the fluctuations in the internal magnetic field due to ion dynamics observed in muon spin relaxation ($$mu$$SR) by an Edwards-Anderson-type autocorrelation function that separates the quasi-static and dynamic components of the correlation by the parameter $$Q$$ (where $$0leq Qleq 1$$). Our Monte Carlo simulations for this model showed that the time evolution of muon spin polarization deviates significantly from the Kubo-Toyabe function. To further validate the model, the results of simulations were compared with the $$mu$$SR spectra observed in a hybrid organic-inorganic perovskite FAPbI$$_3$$ [with FA referring to HC(NH$$_2$$)$$_2$$], where local field fluctuations associated with the rotational motion of FA molecules and quasi-static fields from the PbI$$_3$$ lattice are presumed to coexist. The least-squares curve fitting showed reasonable agreement with the model with $$Q=0.947(3)$$, and the fluctuation frequency of the dynamical component was obtained. This result opens the door to the possibility of experimentally distinguishing fluctuations due to the dynamics of ions around muons from those due to the self-diffusion of muons. On the other hand, it suggests the need to carefully consider the spin relaxation function when applying $$mu$$SR to the issue of ion dynamics.

論文

Effect of dissolved oxygen concentration on dynamic strain aging and stress corrosion cracking of SUS304 stainless steel under high temperature pressurized water

広田 憲亮; 中野 寛子; 藤田 善貴; 武内 伴照; 土谷 邦彦; 出村 雅彦*; 小林 能直*

The IV International Scientific Forum "Nuclear Science and Technologies"; AIP Conference Proceedings 3020, p.030007_1 - 030007_6, 2024/01

沸騰水型原子炉を模擬した高温高圧水中環境下では、溶存酸素量(DO)の変化により動的ひずみ時効(DSA)と粒界型応力腐食割れ(粒界SCC)がそれぞれ発生する。これらの現象の違いを明確に理解するために、その発生メカニズムを整理した。その結果、SUS304ステンレス鋼では、DOが1ppb未満の低濃度では粒内割れによるDSAが発生し、DOが100$$sim$$8500ppbでは表面の酸化膜形成によりDSAは抑制されることがわかった。一方、DOが20000ppbまで上昇すると、皮膜が母材から剥離し、母材の結晶粒界に酸素元素が拡散し、粒界SCCが発生した。これらの結果から、DSAや粒界SCCによるクラック発生を抑制するためには、最適なDO濃度を調整する必要があることが示唆された。

論文

Convergence behavior of statistical uncertainty in probability table for cross section in unresolved resonance region

多田 健一; 遠藤 知弘*

Journal of Nuclear Science and Technology, 60(11), p.1397 - 1405, 2023/11

 被引用回数:1 パーセンタイル:72.91(Nuclear Science & Technology)

確率テーブルは非分離共鳴領域の自己遮蔽効果を取り扱う手法としてよく知られている手法である。確率テーブルの生成には長い計算時間が必要となる。この確率テーブルの生成時間を減らすには、ラダー数を削減することが効果的である。本研究の目的は、確率テーブルの統計誤差を用いて、最適なラダー数を推定することである。そこで本研究では、確率テーブルの統計誤差の定量化方法を開発し、統計誤差の収束挙動を調査した。確率テーブルと平均断面積の積を、統計誤差の指標と見なした。本研究により、統計誤差の収束率は核種ごとに異なっており、統計誤差の収束率は平均レベル間隔と平均中性子幅の影響を受けることが明らかになった。また、入力パラメータをラダー数から統計誤差の許容値に変更した場合、確率テーブルの生成時間が半分以下になることが分かった。

論文

Molecular dynamics analysis of reactor graphite for preparing thermal neutron scattering law

沖田 将一朗; 後藤 実

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 10 Pages, 2023/10

The recently released JENDL-5 and ENDF/B-VIII.0 have adopted porosity-dependent thermal neutron scattering law (TSL) data for reactor graphite, and they improve neutronic calculation accuracy of criticality for graphite-moderated cores. Currently, we can only handle neutronic calculations for three graphite porosities of 0%, 10%, and 30%. The uncertainties associated with the difference between the porosity of actual reactor graphite ($$sim$$20%) and the porosity remains. Toward the future update of JENDL-5, we are planning to preparing new TSL data of reactor graphite. As a first step, it is essential to evalute phonon density state distribution of reactor graphite. In this study, in order to evalute it, molecular dynamic (MD) analysis is performed for three MD models: ideal crystalline graphite (Ideal model), 20%-porous reactor graphite with monoatomic random pore (Monoatomic random model), and 20%-porous reactor graphite with atomic cluster random pore (Cluster random model). The ideal crystalline graphite is modeled without any pores for reference. The 20%-porous reactor graphite with monoatomic random pore is modeled by randomly removing atoms from the ideal crystalline graphite. The 20%-porous reactor graphite with cluster random pore is modeled by randomly removing atomic clusters of approximately 2 nm in diameter from the ideal crystalline graphite. Their interatomic interactions are on the basis of Reactive Empirical Bond Order (REBO) potential. Velocity autocorrelation functions and phonon density of states distributions are calculated for these models. For validation, specific heat for each model is evaluated, and they are compred with experimental values.

論文

Linearization of thermal neutron scattering cross section to optimize the number of energy grid points

多田 健一

Proceedings of 12th International Conference on Nuclear Criticality Safety (ICNC2023) (Internet), 8 Pages, 2023/10

熱中性子散乱則データのエネルギー点数は、連続エネルギーモンテカルロ計算コードの断面ファイルのデータサイズに大きく影響する。エネルギー点数の最適化は、断面ファイルのデータサイズを削減するための効果的な手法の一つである。本研究では、エネルギー点数の最適化のため、熱中性子散乱断面積の線形化機能を開発し、核データ処理コードFRENDYに実装した。線形化手法として、共鳴再構成とドップラー広がりで使用される線形化手法を用いた。エネルギー点数の違いが中性子輸送計算に与える影響を推測するため、ZrHを減速材として用いた臨界実験ベンチマークを計算した。計算結果から、熱中性子断面積の線形化が中性子輸送計算の計算精度が改善することが分かった。

論文

Simulation-based dynamic probabilistic risk assessment of an internal flooding-initiated accident in nuclear power plant using THALES2 and RAPID

久保 光太郎; Zheng, X.; 田中 洋一; 玉置 等史; 杉山 智之; Jang, S.*; 高田 孝*; 山口 彰*

Proceedings of the Institution of Mechanical Engineers, Part O; Journal of Risk and Reliability, 237(5), p.947 - 957, 2023/10

 被引用回数:4 パーセンタイル:69.72(Engineering, Multidisciplinary)

確率論的リスク評価(Probabilistic Risk Assessment: PRA)は、大規模かつ複雑なシステムのリスクを評価するために用いられる手法である。しかし、従来のイベントツリーやフォールトツリーを用いたPRAでは、原子力発電所の構造物、系統及び機器が損傷するタイミングを考慮することは困難である。そこで、この課題を解決するために、RAPID(Risk Assessment with Plant Interactive Dynamics)を用いて、熱水力解析と外部事象のシミュレーションを組み合わせた手法を提案した。加圧水型原子炉のタービン建屋内での内部溢水を表現するために、ベルヌーイの定理に基づいた溢水伝播モデルを適用した。加えて、溢水源の流量や緩和システムの故障基準などの不確実さを考慮した。シミュレーションでは、運転員がいくつか簡略化を行うことにより、運転員による溢水源の隔離操作と排水ポンプを用いた回復操作をモデル化した。その結果、隔離と排水を組み合わせることで、溢水発生時の条件付炉心損傷確率を約90%低減できることが示された。

論文

Solubility of FeSe$$_{2}$$(cr) at 318 K in the presence of iron

吉田 泰*; 北村 暁; 澁谷 早苗*

Journal of Nuclear Science and Technology, 60(8), p.900 - 910, 2023/08

 被引用回数:0 パーセンタイル:0.01(Nuclear Science & Technology)

The concentration of Se equilibrated with FeSe$$_{2}$$(cr) was determined by solubility experiments under reducing conditions and 318 $$pm$$ 1 K. Agreement between the solubility data obtained from the over and under saturation directions suggested the attainment of equilibrium. FeSe$$_{2}$$(cr) phase only formed. The log$$_{10}$$$${it K}$$$$^{0}$$ values of -5.0 $$pm$$ 1.4 and -14.9 $$pm$$ 1.5 for the FeSe$$_{2}$$(cr) solubility reactions respectively were determined. Moreover, the selenium solubility was discussed. At the experimental conditions corresponding to the typical pH and Eh of anoxic groundwater and the equilibrium with stable FeSe$$_{2}$$(cr), the Se solubilities were remained as constant in spite of the linear relationship between iron concentrations with pH. This indicated that Se was consumed before the formation of FeSe$$_{2}$$(cr). This behavior indicated that consideration of reaction paths to equilibrium with FeSe$$_{2}$$(cr) is necessary for an estimation of Se solubility for performance assessment in geological disposal system.

論文

Improvement in the elution performance of an N,N,N',N-tetraoctyl diglycolamide impregnated extraction chromatography adsorbent using neodymium via micro-particle-induced X-ray emission analysis

高畠 容子; 渡部 創; 新井 剛*; 佐藤 隆博*; 柴田 淳広

Applied Radiation and Isotopes, 196, p.110783_1 - 110783_5, 2023/06

 被引用回数:0 パーセンタイル:0.01(Chemistry, Inorganic & Nuclear)

An adsorbent used for the recovery of trivalent minor actinides (MA(III); Am and Cm) from high level liquid waste generated from reprocessing of spent nuclear fuel was subjected to micro-PIXE analysis to improve its elution performance. The experimental adsorbent comprised SiO$$_{2}$$ particles, a polymer coating, and an TODGA. The particles to be analyzed were subjected to Nd adsorption and an elution operation, but Nd in the adsorbent was found to be uniformly distributed. This might have been caused by individual differences in the amount of impregnated TODGA. The remaining Nd species were not localized to a specific part of the adsorbent after the adsorption operation. Some Nd elements were retained in the adsorbent after elution, probably because of the poor diffusion of the mobile phase inside the adsorbent. An adsorbent having a different microstructure from the first was then evaluated, and rapid elution was observed on new adsorbent along micro-PIXE analysis

論文

Development of ACE file perturbation tool using FRENDY

多田 健一; 近藤 諒一; 遠藤 知弘*; 山本 章夫*

Journal of Nuclear Science and Technology, 60(6), p.624 - 631, 2023/06

 被引用回数:2 パーセンタイル:53.91(Nuclear Science & Technology)

感度解析や不確かさ評価は評価済み核データの改良にとって重要な役割を担っている。現在の計算機性能の向上によって、連続エネルギーモンテカルロ計算コードを用いた感度解析や不確かさが可能となってきている。そこで本研究では、FRENDYのモジュールを用いて、連続エネルギーモンテカルロ計算コードで用いられるACEファイルの摂動ツールを開発した。本摂動ツールを用いて微視的断面積,核分裂当たりの中性子数,核分裂スペクトルを摂動させることができる。また、ユーザーが共分散データを用意すれば、ランダムサンプリング法を用いた不確かさ解析を行うこともできる。本摂動ツールの検証のため、実効増倍率の不確かさを感度解析コードSCALE/TSUNAMI及びMCNP/KSENと比較した。その結果、本摂動ツールを用いたランダムサンプリング法で得られた不確かさは、SCALE/TSUNAMIやMCNP/KSENとよく一致することを確認した。

論文

核データ処理に関するIAEA技術者会合に関する報告

多田 健一

核データニュース(インターネット), (135), p.1 - 10, 2023/06

2022年11月29日から12月2日の日程でIAEAが主催したTechnical Meeting on Nuclear Data Processing (核データ処理に関する技術者会合)についての会議の概要を国内の核データ関係者に向けて紹介するものである。本会議では各機関で開発中の核データ処理コードの開発状況や、核データ処理コード間の処理結果などについて報告があった。本稿では、これらの報告内容について詳しく説明する。

論文

Accident sequence precursor analysis of an incident in a Japanese nuclear power plant based on dynamic probabilistic risk assessment

久保 光太郎

Science and Technology of Nuclear Installations, 2023, p.7402217_1 - 7402217_12, 2023/06

 被引用回数:0 パーセンタイル:0.01(Nuclear Science & Technology)

Probabilistic risk assessment (PRA) is an effective methodology that could be used to improve the safety of nuclear power plants in a reasonable manner. Dynamic PRA, as an advanced PRA allows for more realistic and detailed analyses by handling time-dependent information. However, the applications of this method to practical problems are limited because it remains in the research and development stage. This study aimed to investigate the possibility of utilizing dynamic PRA in risk-informed decision-making. Specifically, the author performed an accident sequence precursor (ASP) analysis on the failure of emergency diesel generators that occurred at Unit 1 of the Tomari Nuclear Power Plant in Japan using dynamic PRA. The results were evaluated by comparison with the results of simplified classical PRA. The findings indicated that dynamic PRA may estimate lower risks compared with those obtained from classical PRA by reasonable modeling of alternating current power recovery. The author also showed that dynamic PRA can provide detailed information that cannot be obtained with classical PRA, such as uncertainty distribution of core damage timing and importance measure considering the system failure timing.

論文

Statistical uncertainty quantification of probability tables for unresolved resonance cross sections

多田 健一; 遠藤 知弘*

EPJ Web of Conferences, 284, p.14013_1 - 14013_4, 2023/05

 被引用回数:0 パーセンタイル:0.21(Nuclear Science & Technology)

高速炉及び中速炉では非分離共鳴領域の自己遮蔽効果の影響が大きくなる。確率テーブル法は連続エネルギーモンテカルロ計算コードで非分離共鳴領域の自己遮蔽効果を取り扱う手法として広く利用されている。本手法では、各核種の与えられたエネルギー点において、断面積の確率分布のテーブルを計算している。確率テーブルは、ラダーと呼ばれる疑似共鳴構造を何度も作成し、その平均から計算している。多くの核データ処理コードではこのラダーを作成する回数が入力値として必要となっているが、最適なラダー数は今まで検討されていなかった。以前の著者の研究から、最適なラダー数は核種や平均共鳴パラメータに依存することが分かっている。このことから、核データ処理コードユーザー自身が最適なラダー数を見つけることは困難である。そこで本研究では、確率テーブル生成における統計的不確かさを計算する手法を開発した。開発した手法では、中心極限定理を用いて確率テーブルと平均全断面積の積の統計的不確かさを計算する。

論文

Large-eddy simulation on gas mixing induced by the high-buoyancy flow in the CIGMA facility

安部 諭; 柴本 泰照

Nuclear Engineering and Technology, 55(5), p.1742 - 1756, 2023/05

 被引用回数:0 パーセンタイル:0.01(Nuclear Science & Technology)

The hydrogen behavior in a nuclear containment vessel is a significant issue when discussing the potential of hydrogen combustion during a severe accident. After the Fukushima-Daiichi accident in Japan, we have investigated in-depth the hydrogen transport mechanisms by utilizing experimental and numerical approaches. Computational fluid dynamics is a powerful tool for better understanding the transport behavior of gas mixtures, including hydrogen. This paper describes a large-eddy simulation of gas mixing driven by a high-buoyancy flow. We focused on the interaction behavior of heat and mass transfers driven by the horizontal high-buoyant flow during density stratification. For validation, the experimental data of the Containment InteGral effects Measurement Apparatus (CIGMA) facility were used. With a high-power heater for the gas-injection line in the CIGMA facility, a high temperature flow of approximately 390$$^{circ}$$C was injected into the test vessel. By using the CIGMA facility, we can extend the experimental data to the high temperature region. The phenomenological discussion in this paper help understand the heat and mass transfer induced by the high-buoyancy flow in the containment vessel during a severe accident.

論文

Development of dynamic PRA methodology for external hazards in sodium-cooled fast reactor via applying Markov chain Monte Carlo method to severe accident analysis code; Assessment of accident management of assigning independent emergency diesel generators to each air cooler

Li, C.-Y.; 渡部 晃*; 内堀 昭寛; 岡野 靖

Proceedings of 30th International Conference on Nuclear Engineering (ICONE30) (Internet), 10 Pages, 2023/05

Quantitative assessment of the effect of accident management on the various external hazards is essential in the nuclear safety analysis. This study aims to establish the dynamic probabilistic risk assessment methodology for sodium-cooled fast reactors that can consider the transient plant status under continuous external hazards with corresponding countermeasures operating stochastically. Specifically, the Continuous Markov chain Monte Carlo (CMMC) and Deterministic and Stochastic Petri Nets (DSPN) methods are newly applied to the severe accident analysis code, SPECTRA, which can conduct dynamic plant evaluation in the different severe accident conditions of nuclear reactors, to develop an evaluation methodology for typical external hazards. In the DSPN-CMMC-SPECTRA coupled frame, the latest safety functions of the plant components/systems can be stochastically determined by the DSPN-CMMC grounded on the current plant states under continuous hazard and the interaction between the multi-state components/systems; then, SPECTRA can evaluate the following plant state determined by the latest safety function of the components/systems. Therefore, the advantage of this newly developed DSPN-CMMC-SPECTRA frame is having the capability to quantitatively and stochastically evaluate the transient accident progressions that potentially lead to the core damage under the continuous external hazard scenario. As for the preliminary exam on the DSPN-CMMC-SPECTRA frame, one of the typical external hazards of continuous volcanic ashfall is selected in this research. In addition, the numerical investigation of alternative accident management' effects has also been carried out and quantitatively confirmed in this research.

論文

Dynamic probabilistic risk assessment of seismic-induced flooding in pressurized water reactor by seismic, flooding, and thermal-hydraulics simulations

久保 光太郎; Jang, S.*; 高田 孝*; 山口 彰*

Journal of Nuclear Science and Technology, 60(4), p.359 - 373, 2023/04

 被引用回数:5 パーセンタイル:78.52(Nuclear Science & Technology)

確率論的リスク評価(PRA)は、原子力発電所の安全性を向上させるための重要なアプローチである。しかし、この手法では、複合ハザードのモデル化は困難である。地震に起因した溢水シナリオでは、地震による炉心損傷、溢水による炉心損傷、地震と溢水が組み合わさった炉心損傷といった複数の炉心損傷シーケンスを含んでいる。溢水に係るフラジリティは、溢水がタンクなどの水源から区画に伝播するため、時間依存性を有している。そのため、現実的なリスク評価及び定量化を行うためには、動的リスク評価を用いる必要がある。本研究では、地震,溢水,熱水力シミュレーションを連成させ、複数ハザード間の依存関係を明示的に考慮し、地震起因溢水のリスク評価を行った。特に、福島第一原子力発電所事故を踏まえた安全性向上対策に注目し、システムの耐力に関する感度解析と可搬型ポンプを用いた蒸気発生器代替注水の効果を評価した。我々は、シミュレーションに基づく動的PRA手法の複合ハザード起因のリスクの評価への使用を実証した。

論文

Large-eddy simulation on two-liquid mixing in the horizontal leg and downcomer (the TAMU-CFD Benchmark), with respect to fluctuation behavior of liquid concentration

安部 諭; 岡垣 百合亜

Nuclear Engineering and Design, 404, p.112165_1 - 112165_14, 2023/04

 被引用回数:0 パーセンタイル:0.01(Nuclear Science & Technology)

Pressurized Thermal Shock (PTS) is induced potentially by the rapid cooling of the cold-leg and downcomer wall in the primary system of a Pressurized Water Reactor (PWR) due to the initiation of Emergency Core Cooling System (ECCS). Thus, fluids mixing in a horizontal cold-leg and downcomer should be predicted accurately; however, turbulence production and damping often hinders this prediction due to the presence of the density gradients. Hence, the Fifth International Benchmark Exercise, the cold-leg mixing Computational Fluid Dynamics (CFD) Benchmark, was conducted under the support of OECD/NEA. The experiment was designed for visualization of the mixing phenomena of two liquids with different densities. The heavy liquid was a simulant of cold water from ECCS, in a horizontal leg and downcomer. We used the Large-eddy Simulation (LES) to investigate the time fluctuation behaviors of velocity and liquid concentration. The CFD simulation was performed with two turbulence models and three different numerical meshes. We investigated the characteristics of the appearance frequency of the heavy liquid concentration with the statistical method. Based on our findings, we propose further experiments and numerical investigations to understand the fluid mixing phenomena related to PTS.

論文

Proof-of-principle experiment for testing strong-field quantum electrodynamics with exotic atoms; High precision X-ray spectroscopy of muonic neon

奥村 拓馬*; 橋本 直; 他40名*

Physical Review Letters, 130(17), p.173001_1 - 173001_7, 2023/04

 被引用回数:1 パーセンタイル:83.24(Physics, Multidisciplinary)

To test bound-state quantum electrodynamics (BSQED) in the strong-field regime, we have performed high-precision X-ray spectroscopy of the 5$$g$$-4$$f$$ and 5$$f$$-4$$d$$ transitions (BSQED contribution of 2.4 eV and 5.2 eV, respectively) of muonic neon atoms in the low-pressure gas phase without bound electrons. Muonic atoms have been recently proposed as an alternative to few-electron high-Z ions for BSQED tests by focusing on circular Rydberg states where nuclear contributions are negligibly small. We determined the $$5g_{9/2}$$-$$4f_{7/2}$$ transition energy to be 6297.08 $$pm$$ 0.04 (stat.) $$pm$$ 0.13 (syst.) eV using superconducting transition-edge sensor microcalorimeters (5.2-5.5 eV FWHM resolution), which agrees well with the most advanced BSQED theoretical prediction of 6297.26 eV.

論文

FRENDYで出来ること ※ただし核データ処理を除く

多田 健一

炉物理の研究(インターネット), (75), 13 Pages, 2023/03

FRENDYでは、核データ処理以外にも、核データの編集や断面積データのプロットなど、様々な機能を有している。本資料は核データ処理以外のFRENDYの機能について紹介する。

論文

核データ処理コードFRENDY

多田 健一

遮蔽解析のV&Vガイドライン策定に向けて, p.11 - 16, 2023/03

核データ処理コードFRENDYに詳しくない遮蔽計算コードのユーザーを対象に、FRENDYの概要について紹介する。具体的には、FRENDYでの核データ処理の流れや利用目的、入力例、実施した検証などについて説明する。

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